Energy Dependence of the Isotopic Composition in Nuclear Multifragmentation

Just as a dense liquid, when heated, can exist in an intermediate vapor phase (liquid + gas) before turning into a dilute gas, atomic nuclei too can exist in a mixed phase of heavy fragments and light clusters before dissociating into their constituent nucleons. Unlike ordinary liquid, nuclei is a two component fluid made of neutrons (N) and protons (Z). The two component nature of nuclei can significantly alter the chemical composition of the fragments and the light clusters. In particular, the distillation/fractionation for asymmetric nuclear matter (N/Z > 1) can result in a dilute and neutron rich gas (nucleons and light clusters), and a dense and symmetric liquid (heavy fragments) phase.
The figure on the right shows an experimental evidence of the relative increase in the neutron richness of the light clusters formed in Fe + Ni and Fe + Fe reactions as a function of their N/Z. With increasing N/Z of the system, the excess neutrons are easily available to form neutron rich clusters. With increasing beam energy, the clusters are produced with higher excitation energy, which boils of the excess neutrons making them less neutron rich.